Technique - (9) Terahertz time-domain spectroscopy (THz-TDS)

Type: Experimental

Description: Pulsed THz generation and detection (optical rectification / EO sampling) for broadband dielectric spectroscopy of quantum materials, semiconductors, and biological systems.

Department(s)/lab(s): Imaging Physics (ImPhys) | Adam Lab (THz near-field) @ TU Delft
Summary:

Aurèle Adam develops THz near-field imaging and spectroscopy. Research: (1) apertureless scattering-type near-field optical microscopy (s-SNOM) at THz frequencies for nanometre spatial resolution imaging of material properties; (2) THz time-domain spectroscopy of quantum materials and condensed matter systems; (3) antenna-coupled detectors and sources for THz near-field imaging. Relevant to quantum material characterisation at the nanoscale.

Department(s)/lab(s): Electrical & Electronic Engineering – Photon Science Institute | Boland Group (THz Semiconductor and 2D Materials Spectroscopy) @ Manchester
Summary:

Boland's group focuses on THz spectroscopy of semiconductor nanostructures and 2D materials for quantum sensing applications. Research directions: (1) THz optical pump–THz probe spectroscopy β€” measuring ultrafast carrier dynamics in semiconductor nanowires, quantum wells, and 2D materials (graphene, TMDs, perovskites) after optical excitation; (2) Near-field THz nanoscopy β€” sub-wavelength THz imaging of carrier distributions and quantum phase domains; (3) THz-active quantum devices β€” studying exciton and polaron dynamics in perovskite and III-V semiconductors at THz frequencies; (4) 2D material sensors β€” graphene-based THz detectors and emitters. Applications in quantum-material characterization and quantum sensing.

Department(s)/lab(s): Chemistry – Photon Science Institute | Gardner Group (Analytical and Biomedical Spectroscopy) @ Manchester
Summary:

Gardner's group develops infrared and Raman microspectroscopy for biomedical diagnostics and disease sensing. Research directions: (1) FTIR synchrotron microspectroscopy β€” using Diamond Light Source synchrotron IR beam for high-spatial-resolution chemical mapping of biological tissues for cancer diagnosis; (2) Raman microspectroscopy β€” label-free chemical imaging of cells and tissue for disease classification using machine-learning chemometrics; (3) SERS probes β€” developing gold nanoparticle SERS labels for targeted cancer biomarker detection; (4) Breathomics β€” on-chip photonic sensors for exhaled breath analysis for early disease detection. The infrared and Raman methods provide label-free molecular sensing with potential for quantum-enhanced sensitivity.

Department(s)/lab(s): Physics – Institute for Quantum Electronics | Optical Nanomaterial Group (Grange) @ ETH Zurich
Summary:

Grange leads the Optical Nanomaterial Group at ETH, developing nonlinear materials for quantum photonic integrated circuits. Research directions: (1) Barium titanate (BTO) nanophotonics β€” scalable CMOS-compatible BTO thin-film integrated circuits exploiting large Ο‡(2) nonlinearity for quantum entangled photon-pair generation via SPDC; (2) Lithium niobate on insulator (LNOI) β€” quantum photonic integrated circuits for heralded single-photon sources and electro-optic transduction; (3) Second-harmonic generation sensing β€” SHG-active nanocrystals as contrast agents and phase-sensitive probes in biological imaging; (4) On-chip entangled photon sources for quantum communication and sensing. Strong quantum sensing application in nonlinear optical readout of quantum states.

Department(s)/lab(s): Electrical & Electronic Engineering – Photon Science Institute | Halsall Group (Photonics and Semiconductor Spectroscopy) @ Manchester
Summary:

Halsall is a senior PSI photonics researcher focusing on semiconductor spectroscopy and photonic quantum device characterization. Research directions: (1) Deep-level transient spectroscopy (DLTS) β€” characterizing defects and impurities in semiconductor quantum device structures (Si, GaN, SiC) that are relevant to qubit coherence; (2) Photoluminescence mapping β€” spatial mapping of optical quality in quantum well and dot wafers for quantum sensing device development; (3) InGaN/GaN quantum wells β€” non-destructive optical characterization of LED and sensor structures; (4) THz and infrared spectroscopy β€” contactless Hall measurements and Drude response for quantum material characterization. Provides photonic metrology tools for characterizing quantum sensing device materials.

Department(s)/lab(s): Physics & Astronomy – Photon Science Institute | Hibberd Group (THz Spectroscopy and Quantum Materials) @ Manchester
Summary:

Hibberd holds an EPSRC Ernest Rutherford Fellowship at Manchester's PSI. Research directions: (1) Ultrafast THz spectroscopy of magnetic materials β€” probing spin dynamics, magnon modes, and phase transitions in correlated magnetic materials with sub-ps time resolution using intense THz pulses; (2) THz-driven spintronics β€” using THz electric and magnetic fields to switch magnetization and induce spin currents; (3) THz generation from spintronic heterostructures β€” using ultrafast spin-charge conversion as a broadband THz emitter for materials characterization; (4) Quantum magnonics β€” studying collective spin excitations (magnons) as quantum sensors of materials order parameters. Bridges ultrafast optics and quantum sensing of magnetic phases.

Department(s)/lab(s): School of Physics | Nanophotonics and Electromagnetic Materials Group @ USyd
Summary:

Kuhlmey works on structured electromagnetic materials across an unusually wide frequency range: microstructured optical fibres, metamaterials, non-reciprocal and time-varying media, and β€” the newest and most sensing-relevant thread β€” quantum terahertz photonics, in collaboration with ENS Paris and CSIRO. The THz programme is explicitly aimed at single-photon/single-electron coupling in the THz band, which if it works would allow quantum devices to operate at a few kelvin rather than millikelvin. The group runs a THz time-domain spectroscopy lab with cryogenic capability. Positioned against the established body of NV-ensemble quantum sensing work β€” DEER, nanoscale NMR and T1 relaxometry protocols operating at pT/sqrt(Hz) field sensitivity β€” the THz band is the one part of the spectrum where neither superconducting circuits nor NV ensembles currently offer quantum-limited detection, so this is a genuine gap-filling programme rather than a variation on existing pT/sqrt(Hz) approaches.

Department(s)/lab(s): Department of Chemistry & Applied Biosciences (D-CHAB) – IMPS | Molecular Physics and Spectroscopy Group (Merkt) @ ETH Zurich
Summary:

Merkt leads the Molecular Physics and Spectroscopy group at ETH D-CHAB. Research directions: (1) High-resolution XUV/VUV spectroscopy β€” using synchrotron radiation and table-top laser sources to study molecular Rydberg states, ionization thresholds, and ro-vibrational structure at sub-MHz precision; (2) Precision molecular clock transitions β€” proposing and measuring molecular transitions suitable for fundamental constant variation searches (ΞΌ, Ξ±); (3) Metastable atom and ion trapping β€” developing new trapping methods for precision spectroscopy of exotic species; (4) Pulse and Fourier transform microwave spectroscopy β€” rotational spectroscopy of transient species. Direct applications to molecular quantum sensing and fundamental physics.

Department(s)/lab(s): Physics & Astronomy – Photon Science Institute | Parkinson Group (Ultrafast Spectroscopy of Photonic Materials) @ Manchester
Summary:

Parkinson's group uses ultrafast optical spectroscopy to study carrier dynamics in photonic materials with quantum device applications. Research directions: (1) Time-resolved photoluminescence β€” TRPL with single-photon counting to map exciton lifetimes, diffusion, and defect trapping in GaN, perovskite, and 2D semiconductor quantum wells; (2) Optical single-particle spectroscopy β€” isolating single nanowires or nanocrystals for defect-free measurements of intrinsic optical properties; (3) Photon-number statistics β€” Hanbury Brown–Twiss measurements of single-photon purity from quantum dots and localized excitons; (4) Semiconductor quantum sensing interfaces β€” studying how carrier dynamics affect the fidelity of semiconductor-based quantum sensors and emitters.