Technique - (5) Synchrotron X-ray fluorescence microscopy

Type: Experimental

Description: Nanoscale elemental mapping using focused synchrotron X-ray beams at facilities such as the Advanced Photon Source.

Department(s)/lab(s): Physics – Laboratory for Solid State Physics (ETH) / PSI / EPFL | Quantum Technologies Group (Aeppli, ETH/PSI/EPFL) @ ETH Zurich
Summary:

Aeppli leads the Quantum Technologies Group spanning ETH Zurich, EPFL, and PSI. Research directions: (1) Quantum materials imaging — using SLS synchrotron X-rays (including SwissFEL ultrafast pulses) and neutrons at SINQ to image quantum phase transitions, skyrmions, and correlated phases; non-destructive imaging of device structures; (2) Rare-earth quantum magnets and qubits — LiHoF4 as a model quantum system; Er, Pr, and Nd spin qubits in crystals for quantum information and sensing; (3) Semiconductor quantum devices — silicon and germanium nanostructures probed by synchrotron nanoscale X-ray imaging; (4) Van der Waals materials and CDW memory devices. Strong interface with PSI large-scale facilities as unique quantum sensing tools for materials.

Department(s)/lab(s): School of Physics | Chantler X-ray and Precision Atomic Physics Group @ UMelb
Summary:

Chantler's group is built around the idea that X-ray measurements can be made accurate, not just precise: the X-ray Extended Range Technique (XERT) delivers absolute absorption coefficients at the 0.02 per cent level, which in turn allows XAFS to be used for quantitative structure determination and allows high-accuracy tests of atomic theory. The second thread is precision X-ray spectroscopy of highly charged ions and exotic atoms as a test of bound-state QED, where discrepancies between theory and experiment remain unresolved. Positioned against the established body of NV-ensemble quantum sensing work — DEER, nanoscale NMR and T1 relaxometry protocols operating at pT/sqrt(Hz) field sensitivity — this is precision measurement at the other end of the electromagnetic spectrum: the methodological common ground with pT/sqrt(Hz) NV ensemble sensing is the obsessive treatment of systematics and absolute calibration that separates a sensitive measurement from an accurate one. Borderline inclusion, kept because the group's core competency is metrology rather than X-ray applications.

Department(s)/lab(s): Department of Materials (D-MATL) | Magnetism and Interface Physics Group (Gambardella) @ ETH Zurich
Summary:

Gambardella leads the Magnetism and Interface Physics group at ETH D-MATL. Research directions: (1) Scanning probe magnetometry — using NV-center cantilevers (collaboration with Degen) and magneto-optical Kerr microscopy to image spin textures (skyrmions, domain walls) in thin-film heterostructures with sub-100 nm resolution; (2) Spin-orbit torques — current-induced magnetization switching via interfacial spin-orbit coupling; spin Hall and Rashba effects for spintronic devices; (3) Single-atom magnetism — STM and X-ray absorption for element-specific orbital and spin moments of individual atoms on surfaces; (4) XMCD at synchrotron — quantitative element-specific magnetic spectroscopy. Quantum sensing angle: spin-orbit driven phenomena, high-resolution magnetic imaging.

Department(s)/lab(s): Physics | Pupa Gilbert Research Group @ UWMadison
Summary:

Uses X-ray photoemission electron microscopy (X-PEEM) with XANES spectroscopy at synchrotron light sources to map crystal orientation and amorphous-to-crystalline transitions at ~10 nm resolution in biominerals (coral skeletons, sea urchin spines, mollusk nacre, tooth enamel).

Department(s)/lab(s): Physics and Astronomy | Jacobsen Research Group (X-ray Microscopy) @ Northwestern
Summary:

Prof. Jacobsen's group develops novel methods, instruments, and analysis approaches for X-ray nanoscale imaging and applies them to biology and environmental science, using the Advanced Photon Source (APS) at Argonne. Directions: (1) Scanning X-ray fluorescence microscopy (SXFM) for organ-wide and nanoscale elemental mapping of metals (zinc, copper, iron) in biological tissues — central to the NIH-funded QE-Map national resource; imaging how metals regulate cellular functions, synaptic zinc signaling, and neurodegenerative disease; (2) X-ray ptychography and coherent diffractive imaging (CDI) for nanoscale biological imaging beyond the diffraction limit with improved dose efficiency; (3) Development of new algorithms, optics (zone plates), and detector systems to push spatial resolution and dose efficiency in X-ray microscopy — including lensless imaging methods and compressed-sensing reconstruction. Joint appointment at Argonne National Laboratory (Argonne Distinguished Fellow); also involved in QE-Map resource with Kozorovitskiy and Hao Zhang (McCormick).