Technique - (13) Time-resolved photoluminescence (TRPL) and single-photon counting

Type: Experimental

Description: Pulsed excitation with TCSPC or streak camera detection for carrier lifetime, exciton dynamics, and defect characterization in photonic materials and quantum dots.

Department(s)/lab(s): Physics & Astronomy – Photon Science Institute | Parkinson Group (Ultrafast Spectroscopy of Photonic Materials) @ Manchester
Summary:

Parkinson's group uses ultrafast optical spectroscopy to study carrier dynamics in photonic materials with quantum device applications. Research directions: (1) Time-resolved photoluminescence β€” TRPL with single-photon counting to map exciton lifetimes, diffusion, and defect trapping in GaN, perovskite, and 2D semiconductor quantum wells; (2) Optical single-particle spectroscopy β€” isolating single nanowires or nanocrystals for defect-free measurements of intrinsic optical properties; (3) Photon-number statistics β€” Hanbury Brown–Twiss measurements of single-photon purity from quantum dots and localized excitons; (4) Semiconductor quantum sensing interfaces β€” studying how carrier dynamics affect the fidelity of semiconductor-based quantum sensors and emitters.

Department(s)/lab(s): School of Chemistry | Smith Time-Resolved Spectroscopy and Microspectroscopy Group @ UMelb
Summary:

Smith runs Melbourne's time-resolved fluorescence facility and specialises in the information channels most people throw away: fluorescence lifetime, anisotropy decay and its orientational content, and single-molecule photophysics, applied to organic semiconductors, energy-transfer systems and biological samples. The group builds its own confocal microspectroscopy instrumentation for time-resolved anisotropy imaging and single-molecule detection. Positioned against the established body of NV-ensemble quantum sensing work β€” DEER, nanoscale NMR and T1 relaxometry protocols operating at pT/sqrt(Hz) field sensitivity β€” lifetime- and orientation-resolved fluorescence is the principal orthogonal contrast mechanism to spin-based sensing, and his instrumentation is the natural correlative partner for NV-ensemble DEER/relaxometry experiments at pT/sqrt(Hz) that need an independent optical readout of the same specimen. Preferred attribute present: orientation- and lifetime-resolved methods.

Department(s)/lab(s): Physics & Astronomy | Zheltikov Biophotonics Laboratory @ TAMU
Summary:

Zheltikov integrates NV-diamond magnetometry into photonic-crystal fibers for high-resolution, fiber-delivered magnetic-field imaging and endoscopy, alongside ultrafast biophotonics (multiphoton deep-tissue imaging, SWIR probes) and quantum-light molecular spectroscopy. In the broader landscape of NV-centre ensemble quantum sensing (DEER, nano-NMR, T1 relaxometry) operating near pT/sqrt(Hz) sensitivity, this work extends NV ensemble sensing into fiberized, in-vivo-compatible geometries.