Tarbutt co-leads the Imperial eEDM experiment using YbF molecules and runs an independent molecular array quantum computing/sensing programme. Two parallel eEDM experiments: (1) Ultracold YbF beam — 2D transverse laser cooling producing 200 μK, 2×10^5 molecules/shot, eEDM sensitivity of 1.8×10^−28 e·cm/day (near shot-noise limit); (2) YbF 3D optical lattice — aiming for 10^−30 e·cm/year, requires laser cooling to μK and loading into 3D optical lattice, using novel all-optical spin polarisation and analysis. Also leads UKRI project on testing fundamental physics using arrays of ultracold molecules (CaF in optical tweezers for two-qubit molecular gates). These experiments probe CP-violation and BSM physics at PeV energy scales through precision molecular spectroscopy.